Moment of inertia, backbending, and molecular bifurcation.
نویسندگان
چکیده
We predict an anomaly in highly excited bending spectra of acetylene with high vibrational angular momentum. We interpret this in terms of a vibrational shape effect with moment of inertia backbending, induced by a sequence of bifurcations with a transition from "local" to "orthogonal" modes.
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عنوان ژورنال:
- The Journal of chemical physics
دوره 127 4 شماره
صفحات -
تاریخ انتشار 2007